A one-pot synthesis of multifunctional Bi


Journal

Journal of materials chemistry. B
ISSN: 2050-7518
Titre abrégé: J Mater Chem B
Pays: England
ID NLM: 101598493

Informations de publication

Date de publication:
14 05 2020
Historique:
pubmed: 7 4 2020
medline: 1 5 2021
entrez: 7 4 2020
Statut: ppublish

Résumé

As a direct thin band gap n-type semiconductor, bismuth sulfide (Bi2S3) nanomaterials possess great near-infrared (NIR)-triggered photothermal effects, photoacoustic (PA) and computed tomography (CT) imaging properties. Hence, Bi2S3 nanomaterials have become a research focal point in multiple domains, such as the construction of NIR-triggered nanosystems for cancer therapy. In this study, through a simple one-pot synthesis with the assistance of EDTA-2Na, we first obtained monodispersed spherical Bi2S3 of uniform particle sizes with fascinating photothermal and PA/CT imaging properties. Based on this, we introduced the photosensitizer Ce6 with photodynamic property and CeO2 with the O2-evolving characteristic, and thus designed a core-shell structure of the Bi2S3@Ce6-CeO2 nanocomposites (Bi2S3@Ce6-CeO2 NCs). The as-received Bi2S3@Ce6-CeO2 NCs exhibited a remarkable synergetic photothermal and photodynamic therapeutic effect both in vitro and in vivo, demonstrating its promising potential for cancer treatments. In the long term, the multifunctional PA/CT properties of both Bi2S3 NPs and Bi2S3@Ce6-CeO2 NCs in this study also supply a novel Bi2S3-based platform for constructing integrated diagnosis and treatment platforms.

Identifiants

pubmed: 32249879
doi: 10.1039/d0tb00080a
doi:

Substances chimiques

Antineoplastic Agents 0
Biocompatible Materials 0
Photosensitizing Agents 0
Sulfides 0
Cerium 30K4522N6T
ceric oxide 619G5K328Y
Bismuth U015TT5I8H
bismuth sulfide XZC47M60X8

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

4093-4105

Auteurs

Lingwan Zeng (L)

National Engineering Research Center for Biomaterials, Sichuan University, Chengdu, 610064, China. hsfan@scu.edu.cn.

Huan Zhao (H)

National Engineering Research Center for Biomaterials, Sichuan University, Chengdu, 610064, China. hsfan@scu.edu.cn.

Yuda Zhu (Y)

National Engineering Research Center for Biomaterials, Sichuan University, Chengdu, 610064, China. hsfan@scu.edu.cn.

Suping Chen (S)

National Engineering Research Center for Biomaterials, Sichuan University, Chengdu, 610064, China. hsfan@scu.edu.cn.

Yusheng Zhang (Y)

National Engineering Research Center for Biomaterials, Sichuan University, Chengdu, 610064, China. hsfan@scu.edu.cn.

Dan Wei (D)

National Engineering Research Center for Biomaterials, Sichuan University, Chengdu, 610064, China. hsfan@scu.edu.cn.

Jing Sun (J)

National Engineering Research Center for Biomaterials, Sichuan University, Chengdu, 610064, China. hsfan@scu.edu.cn.

Hongsong Fan (H)

National Engineering Research Center for Biomaterials, Sichuan University, Chengdu, 610064, China. hsfan@scu.edu.cn.

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Classifications MeSH