Ammonium Sulfate to Modulate Crystallization for High-Performance Rigid and Flexible Perovskite Solar Cells.
charge carrier dynamics
defect passivation
multifunctional additives
perovskite solar cells
stability
Journal
Small (Weinheim an der Bergstrasse, Germany)
ISSN: 1613-6829
Titre abrégé: Small
Pays: Germany
ID NLM: 101235338
Informations de publication
Date de publication:
01 May 2024
01 May 2024
Historique:
revised:
10
04
2024
received:
01
03
2024
medline:
2
5
2024
pubmed:
2
5
2024
entrez:
1
5
2024
Statut:
aheadofprint
Résumé
Perovskite solar cells (PSCs) are attracting widespread research and attention as highly promising candidates in the field of electronic photovoltaics owing to their exceptional power conversion efficiency (PCE). However, rigid or flexible PSCs still face challenges in preparing full-coverage and low-defect perovskite films, as well as achieving highly reproducible and highly stable devices. Herein, a multifunctional additive 2-aminoethyl hydrogen sulfate (AES) is designed to regulate the film crystallization and thereby form flat and pinhole-free perovskite films. It is found that the introduction of AES can effectively passivate defects, restrain charge carrier recombination, and then achieve a higher fill factor. As seen with grazing incidence wide-angle X-ray scattering (GIWAXS), this approach does not affect the crystal orientation distribution. It is observed that AES addition shows a universality across different perovskite components since the PCE is improved up to 20.7% for FA
Identifiants
pubmed: 38693078
doi: 10.1002/smll.202401456
doi:
Types de publication
Journal Article
Langues
eng
Sous-ensembles de citation
IM
Pagination
e2401456Subventions
Organisme : Deutsche Forschungsgemeinschaft
ID : EXC2089/1-390776260
Organisme : Deutsche Forschungsgemeinschaft
ID : IRTG2022
Organisme : Bayerisches Staatsministerium für Wissenschaft und Kunst
ID : SolTech
Organisme : Center for NanoScience (CeNS)
Organisme : China Scholarship Council (CSC)
Informations de copyright
© 2024 The Authors. Small published by Wiley‐VCH GmbH.
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