Design of Microchannel Suitable for Packing with Anion Exchange Resins: Uranium Separation from Seawater Containing a Large Amount of Cesium.

Resin-packed microchannel design of microchannel inductively coupled plasma mass spectrometry seawater uranium separation

Journal

Analytical sciences : the international journal of the Japan Society for Analytical Chemistry
ISSN: 1348-2246
Titre abrégé: Anal Sci
Pays: Switzerland
ID NLM: 8511078

Informations de publication

Date de publication:
10 Dec 2021
Historique:
pubmed: 27 7 2021
medline: 15 12 2021
entrez: 26 7 2021
Statut: ppublish

Résumé

We present a resin-packed microchannel that can reduce the radiation exposure risk and secondary radioactive wastes during uranium (U) separation by downscaling the separation using a microchip. Two types of microchips were designed to densely pack the microchannels with resins. The microchannels had almost the same cross-sectional area, but different outer circumferences. A satisfactory separation performance could be obtained by arranging more than ca. 10 resins along the depth and width of the microchannels. A resin-packed microchannel is an effective separation technique for determining the U concentration via inductively coupled plasma mass spectrometry owing to its ability to avoid the contamination of equipment by cesium, and to reduce the matrix effect. The size of the separation site was scaled down to <1/5000 compared to commonly used counterparts. The radiation exposure risk and secondary radioactive wastes can be reduced by 10- and 800-fold, respectively, using a resin-packed microchannel.

Identifiants

pubmed: 34305053
doi: 10.2116/analsci.21P110
pii: 10.2116/analsci.21P110
doi:

Substances chimiques

Anion Exchange Resins 0
Cesium 1KSV9V4Y4I
Uranium 4OC371KSTK

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

1789-1794

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Auteurs

Kazuki Ouchi (K)

Nuclear Science and Engineering Center, Japan Atomic Energy Agency, 2-4 Shirakata, Tokai-mura, Naka, Ibaraki, 319-1195, Japan. ouchi.kazuki@jaea.go.jp.

Takehiko Tsukahara (T)

Laboratory for Advanced Nuclear Energy, Institute of Innovative Research, Tokyo Institute of Technology, 2-12-1-N1-6 O-okayama, Meguro, Tokyo, 152-8550, Japan.

Aileen Brandt (A)

Laboratory for Advanced Nuclear Energy, Institute of Innovative Research, Tokyo Institute of Technology, 2-12-1-N1-6 O-okayama, Meguro, Tokyo, 152-8550, Japan.

Yoshiki Muto (Y)

Laboratory for Advanced Nuclear Energy, Institute of Innovative Research, Tokyo Institute of Technology, 2-12-1-N1-6 O-okayama, Meguro, Tokyo, 152-8550, Japan.

Nozomi Nabatame (N)

Graduate School of Science and Engineering, Ibaraki University, 2-1-1 Bunkyo, Mito, Ibaraki, 310-8512, Japan.

Yoshihiro Kitatsuji (Y)

Nuclear Science and Engineering Center, Japan Atomic Energy Agency, 2-4 Shirakata, Tokai-mura, Naka, Ibaraki, 319-1195, Japan.

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