Stalling chromophore synthesis of the fluorescent protein Venus reveals the molecular basis of the final oxidation step.


Journal

Chemical science
ISSN: 2041-6520
Titre abrégé: Chem Sci
Pays: England
ID NLM: 101545951

Informations de publication

Date de publication:
31 Mar 2021
Historique:
entrez: 25 6 2021
pubmed: 26 6 2021
medline: 26 6 2021
Statut: epublish

Résumé

Fluorescent proteins (FPs) have revolutionised the life sciences, but the mechanism of chromophore maturation is still not fully understood. Here we show that incorporation of a photo-responsive non-canonical amino acid within the chromophore stalls maturation of Venus, a yellow FP, at an intermediate stage; a crystal structure indicates the presence of O

Identifiants

pubmed: 34168826
doi: 10.1039/d0sc06693a
pii: d0sc06693a
pmc: PMC8188506
doi:

Types de publication

Journal Article

Langues

eng

Pagination

7735-7745

Subventions

Organisme : Biotechnology and Biological Sciences Research Council
ID : BB/H003746/1
Pays : United Kingdom

Informations de copyright

This journal is © The Royal Society of Chemistry.

Déclaration de conflit d'intérêts

There are no conflicts to declare.

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Auteurs

Husam Sabah Auhim (HS)

School of Biosciences, Molecular Biosciences Division, Cardiff University Sir Martin Evans Building Cardiff CF10 3AX UK jonesdd@cardiff.ac.uk +44 (0)29 2087 4290.
Department of Biology, College of Science, University of Baghdad Baghdad Iraq.

Bella L Grigorenko (BL)

Chemistry Department, Lomonosov Moscow State University Leninskie Gory, 1-3 Moscow Russian Federation anem@lcc.chem.msu.ru +7 495 939 1096.
Emanuel Institute of Biochemical Physics, Russian Academy of Sciences Moscow Russian Federation.

Tessa K Harris (TK)

School of Biosciences, Molecular Biosciences Division, Cardiff University Sir Martin Evans Building Cardiff CF10 3AX UK jonesdd@cardiff.ac.uk +44 (0)29 2087 4290.

Ozan E Aksakal (OE)

School of Biosciences, Molecular Biosciences Division, Cardiff University Sir Martin Evans Building Cardiff CF10 3AX UK jonesdd@cardiff.ac.uk +44 (0)29 2087 4290.

Igor V Polyakov (IV)

Chemistry Department, Lomonosov Moscow State University Leninskie Gory, 1-3 Moscow Russian Federation anem@lcc.chem.msu.ru +7 495 939 1096.
Emanuel Institute of Biochemical Physics, Russian Academy of Sciences Moscow Russian Federation.

Colin Berry (C)

School of Biosciences, Molecular Biosciences Division, Cardiff University Sir Martin Evans Building Cardiff CF10 3AX UK jonesdd@cardiff.ac.uk +44 (0)29 2087 4290.

Gabriel Dos Passos Gomes (GDP)

Department of Chemistry, University of Toronto 80 St. George Street Toronto ON M5S 3H6 Canada.
Department of Computer Science, University of Toronto 214 College St. Toronto Ontario M5T 3A1 Canada.

Igor V Alabugin (IV)

Department of Chemistry and Biochemistry, Florida State University Tallahassee Fl 32306 USA alabugin@chem.fsu.edu +1 850 644 5795.

Pierre J Rizkallah (PJ)

School of Medicine, Cardiff University CF14 4XN UK.

Alexander V Nemukhin (AV)

Chemistry Department, Lomonosov Moscow State University Leninskie Gory, 1-3 Moscow Russian Federation anem@lcc.chem.msu.ru +7 495 939 1096.
Emanuel Institute of Biochemical Physics, Russian Academy of Sciences Moscow Russian Federation.

D Dafydd Jones (DD)

School of Biosciences, Molecular Biosciences Division, Cardiff University Sir Martin Evans Building Cardiff CF10 3AX UK jonesdd@cardiff.ac.uk +44 (0)29 2087 4290.

Classifications MeSH