The Formation of Mn-Ce Oxide Catalysts for CO Oxidation by Oxalate Route: The Role of Manganese Content.

CO oxidation ceria manganese oxide nanostructure solid solution

Journal

Nanomaterials (Basel, Switzerland)
ISSN: 2079-4991
Titre abrégé: Nanomaterials (Basel)
Pays: Switzerland
ID NLM: 101610216

Informations de publication

Date de publication:
12 Apr 2021
Historique:
received: 15 03 2021
revised: 02 04 2021
accepted: 07 04 2021
entrez: 30 4 2021
pubmed: 1 5 2021
medline: 1 5 2021
Statut: epublish

Résumé

The Mn-Ce oxide catalysts active in the oxidation of CO were studied by X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS), temperature-programmed reduction (TPR), transition electron microscopy (TEM), energy dispersive X-Ray (EDX), and a differential dissolution technique. The Mn-Ce catalysts were prepared by thermal decomposition of oxalates by varying the Mn:Ce ratio. The nanocrystalline oxides with a fluorite structure and particle sizes of 4-6 nm were formed. The introduction of manganese led to a reduction of the oxide particle size, a decrease in the surface area, and the formation of a Mn

Identifiants

pubmed: 33921273
pii: nano11040988
doi: 10.3390/nano11040988
pmc: PMC8070498
pii:
doi:

Types de publication

Journal Article

Langues

eng

Subventions

Organisme : Russian Science Foundation
ID : 19-73-00097

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Auteurs

Olga A Bulavchenko (OA)

Boreskov Institute of Catalysis SB RAS, Lavrentiev Ave. 5, 630090 Novosibirsk, Russia.

Tatyana N Afonasenko (TN)

Center of New Chemical Technologies BIC, Boreskov Institute of Catalysis, Neftezavodskaya 54, 644040 Omsk, Russia.

Alexey R Osipov (AR)

Center of New Chemical Technologies BIC, Boreskov Institute of Catalysis, Neftezavodskaya 54, 644040 Omsk, Russia.

Alena A Pochtar' (AA)

Boreskov Institute of Catalysis SB RAS, Lavrentiev Ave. 5, 630090 Novosibirsk, Russia.

Andrey A Saraev (AA)

Boreskov Institute of Catalysis SB RAS, Lavrentiev Ave. 5, 630090 Novosibirsk, Russia.

Zahar S Vinokurov (ZS)

Boreskov Institute of Catalysis SB RAS, Lavrentiev Ave. 5, 630090 Novosibirsk, Russia.

Evgeny Yu Gerasimov (EY)

Boreskov Institute of Catalysis SB RAS, Lavrentiev Ave. 5, 630090 Novosibirsk, Russia.

Sergey V Tsybulya (SV)

Boreskov Institute of Catalysis SB RAS, Lavrentiev Ave. 5, 630090 Novosibirsk, Russia.

Classifications MeSH