Tuning ferromagnetism at room temperature by visible light.

CH3NH3PbI3 LSMO heat-assisted magnetic recording magnetism tuning

Journal

Proceedings of the National Academy of Sciences of the United States of America
ISSN: 1091-6490
Titre abrégé: Proc Natl Acad Sci U S A
Pays: United States
ID NLM: 7505876

Informations de publication

Date de publication:
24 Mar 2020
Historique:
pubmed: 11 3 2020
medline: 11 3 2020
entrez: 11 3 2020
Statut: ppublish

Résumé

Most digital information today is encoded in the magnetization of ferromagnetic domains. The demand for ever-increasing storage space fuels continuous research for energy-efficient manipulation of magnetism at smaller and smaller length scales. Writing a bit is usually achieved by rotating the magnetization of domains of the magnetic medium, which relies on effective magnetic fields. An alternative approach is to change the magnetic state directly by acting on the interaction between magnetic moments. Correlated oxides are ideal materials for this because the effects of a small external control parameter are amplified by the electronic correlations. Here, we present a radical method for reversible, light-induced tuning of ferromagnetism at room temperature using a halide perovskite/oxide perovskite heterostructure. We demonstrate that photoinduced charge carriers from the [Formula: see text] photovoltaic perovskite efficiently dope the thin [Formula: see text] film and decrease the magnetization of the ferromagnetic state, allowing rapid rewriting of the magnetic bit. This manipulation could be accomplished at room temperature; hence this opens avenues for magnetooptical memory devices.

Identifiants

pubmed: 32152127
pii: 1915370117
doi: 10.1073/pnas.1915370117
pmc: PMC7104399
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

6417-6423

Déclaration de conflit d'intérêts

The authors declare no competing interest.

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Auteurs

Bálint Náfrádi (B)

Laboratory of Physics of Complex Matter, Ecole Polytechnique Fédérale de Lausanne, CH-1015 Lausanne, Switzerland; laszlo.forro@epfl.ch nafradi@yahoo.com.

Péter Szirmai (P)

Laboratory of Physics of Complex Matter, Ecole Polytechnique Fédérale de Lausanne, CH-1015 Lausanne, Switzerland.

Massimo Spina (M)

Laboratory of Physics of Complex Matter, Ecole Polytechnique Fédérale de Lausanne, CH-1015 Lausanne, Switzerland.

Andrea Pisoni (A)

Laboratory of Physics of Complex Matter, Ecole Polytechnique Fédérale de Lausanne, CH-1015 Lausanne, Switzerland.

Xavier Mettan (X)

Laboratory of Physics of Complex Matter, Ecole Polytechnique Fédérale de Lausanne, CH-1015 Lausanne, Switzerland.

Norbert M Nemes (NM)

GFMC, Departamento de Fisica de Materiales, Universidad Complutense de Madrid, 28040 Madrid, Spain.
Unidad Asociada ICMM-CSIC "Laboratorio de Heteroestructuras con Aplicacion en Espintronica," Consejo Superior de Investigaciones Cientificas, 28049 Madrid, Spain.

László Forró (L)

Laboratory of Physics of Complex Matter, Ecole Polytechnique Fédérale de Lausanne, CH-1015 Lausanne, Switzerland; laszlo.forro@epfl.ch nafradi@yahoo.com.

Endre Horváth (E)

Laboratory of Physics of Complex Matter, Ecole Polytechnique Fédérale de Lausanne, CH-1015 Lausanne, Switzerland.

Classifications MeSH