Titania supported synergistic palladium single atoms and nanoparticles for room temperature ketone and aldehydes hydrogenation.

Journal

Nature communications
ISSN: 2041-1723
Titre abrégé: Nat Commun
Pays: England
ID NLM: 101528555

Informations de publication

Date de publication:
07 Jan 2020
Historique:
received: 05 05 2019
accepted: 09 12 2019
entrez: 9 1 2020
pubmed: 9 1 2020
medline: 9 1 2020
Statut: epublish

Résumé

Selective reduction of ketone/aldehydes to alcohols is of great importance in green chemistry and chemical engineering. Highly efficient catalysts are still demanded to work under mild conditions, especially at room temperature. Here we present a synergistic function of single-atom palladium (Pd

Identifiants

DOI: 10.1038/s41467-019-13941-5 PMID: 31911600 PMC: PMC6946645
pubmed: 31911600
doi: 10.1038/s41467-019-13941-5
pii: 10.1038/s41467-019-13941-5
pmc: PMC6946645
doi:

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

48

Références

J Am Chem Soc. 2015 Aug 26;137(33):10484-7
pubmed: 26268551
Nat Mater. 2019 Jul;18(7):746-751
pubmed: 31011216
Chem Commun (Camb). 2014 Jun 7;50(45):6049-51
pubmed: 24769812
Phys Chem Chem Phys. 2014 Oct 21;16(39):21446-51
pubmed: 25183457
J Am Chem Soc. 2017 Jun 21;139(24):8078-8081
pubmed: 28595012
Phys Rev Lett. 1996 Oct 28;77(18):3865-3868
pubmed: 10062328
Chemistry. 2019 Dec 5;25(68):15586-15593
pubmed: 31574171
Chem Rev. 2017 Sep 13;117(17):11522-11569
pubmed: 28872309
ACS Appl Mater Interfaces. 2015 Apr 1;7(12):6480-9
pubmed: 25785883
Proc Natl Acad Sci U S A. 2018 Mar 20;115(12):2902-2907
pubmed: 29507243
Nat Commun. 2014 Dec 03;5:5634
pubmed: 25465918
J Am Chem Soc. 2016 May 25;138(20):6396-9
pubmed: 27167705
Phys Rev B Condens Matter. 1991 Jul 15;44(3):943-954
pubmed: 9999600
J Phys Chem Lett. 2016 Feb 4;7(3):480-5
pubmed: 26747698
Science. 2014 Dec 19;346(6216):1498-501
pubmed: 25431492
Chem Commun (Camb). 2011 Nov 7;47(41):11546-8
pubmed: 21952644
J Comput Chem. 2006 Nov 30;27(15):1787-99
pubmed: 16955487
J Am Chem Soc. 2017 Jul 19;139(28):9419-9422
pubmed: 28661130
Acc Chem Res. 2013 Aug 20;46(8):1740-8
pubmed: 23815772
Phys Rev Lett. 2009 Dec 11;103(24):246102
pubmed: 20366214
J Am Chem Soc. 2018 Jun 20;140(24):7407-7410
pubmed: 29863867
Nat Chem. 2011 Jul 22;3(8):634-41
pubmed: 21778984
Chem Rev. 2012 May 9;112(5):2714-38
pubmed: 22324402
Science. 2010 Sep 24;329(5999):1633-6
pubmed: 20929844
J Am Chem Soc. 2006 Apr 12;128(14):4510-1
pubmed: 16594653
Science. 2016 May 13;352(6287):797-801
pubmed: 27174982
J Synchrotron Radiat. 2005 Jul;12(Pt 4):537-41
pubmed: 15968136
Chem Soc Rev. 2015 Apr 7;44(7):1861-85
pubmed: 25590565
Nat Mater. 2013 Jun;12(6):562-8
pubmed: 23644521
J Am Chem Soc. 2017 May 31;139(21):7294-7301
pubmed: 28502173
Nat Nanotechnol. 2018 Sep;13(9):856-861
pubmed: 30013217
J Am Chem Soc. 2018 Jan 24;140(3):954-962
pubmed: 29262678

Auteurs

Long Kuai (L)

College of Chemistry and Materials Science, The Key Laboratory of Functional Molecular Solids, Ministry of Education, Anhui Laboratory of Molecular-Based Materials, The Key Laboratory of Electrochemical Clean Energy of Anhui Higher Education Institutes, Anhui Normal University, No. 189 South Jiuhua Road, Wuhu, 241002, P. R. China.
School of Chemical and Biological Engineering, Anhui Polytechnic University, Beijing Middle Road, Wuhu, 241000, China.

Zheng Chen (Z)

Department of Chemistry, Tsinghua University, Beijing, 100084, China.
ORCID: 0000-0002-4347-0235

Shoujie Liu (S)

College of Chemistry and Materials Science, The Key Laboratory of Functional Molecular Solids, Ministry of Education, Anhui Laboratory of Molecular-Based Materials, The Key Laboratory of Electrochemical Clean Energy of Anhui Higher Education Institutes, Anhui Normal University, No. 189 South Jiuhua Road, Wuhu, 241002, P. R. China.

Erjie Kan (E)

School of Chemical and Biological Engineering, Anhui Polytechnic University, Beijing Middle Road, Wuhu, 241000, China.

Nan Yu (N)

College of Chemistry and Materials Science, The Key Laboratory of Functional Molecular Solids, Ministry of Education, Anhui Laboratory of Molecular-Based Materials, The Key Laboratory of Electrochemical Clean Energy of Anhui Higher Education Institutes, Anhui Normal University, No. 189 South Jiuhua Road, Wuhu, 241002, P. R. China.

Yiming Ren (Y)

School of Chemical and Biological Engineering, Anhui Polytechnic University, Beijing Middle Road, Wuhu, 241000, China.

Caihong Fang (C)

College of Chemistry and Materials Science, The Key Laboratory of Functional Molecular Solids, Ministry of Education, Anhui Laboratory of Molecular-Based Materials, The Key Laboratory of Electrochemical Clean Energy of Anhui Higher Education Institutes, Anhui Normal University, No. 189 South Jiuhua Road, Wuhu, 241002, P. R. China.

Xingyang Li (X)

School of Chemical and Biological Engineering, Anhui Polytechnic University, Beijing Middle Road, Wuhu, 241000, China.

Yadong Li (Y)

Department of Chemistry, Tsinghua University, Beijing, 100084, China. ydli@tsinghua.edu.cn.

Baoyou Geng (B)

College of Chemistry and Materials Science, The Key Laboratory of Functional Molecular Solids, Ministry of Education, Anhui Laboratory of Molecular-Based Materials, The Key Laboratory of Electrochemical Clean Energy of Anhui Higher Education Institutes, Anhui Normal University, No. 189 South Jiuhua Road, Wuhu, 241002, P. R. China. bygeng@mail.ahnu.edu.cn.

Classifications MeSH