Paramagnetic Lanthanide NMR Probes Signalling Changes in Zinc Concentration by Emission and Chemical Shift: A Proof of Concept Study.

NMR emission lanthanides paramagnetic zinc

Journal

Chemistry (Weinheim an der Bergstrasse, Germany)
ISSN: 1521-3765
Titre abrégé: Chemistry
Pays: Germany
ID NLM: 9513783

Informations de publication

Date de publication:
26 Apr 2019
Historique:
received: 08 02 2019
revised: 08 03 2019
pubmed: 13 3 2019
medline: 13 3 2019
entrez: 13 3 2019
Statut: ppublish

Résumé

A zinc-selective probe based on a set of rare earth complexes of a modified DO3A macrocyclic ligand incorporating a tris-pyridylamine (TPA) moiety has been structurally characterised in solution and in the solid-state. One pyridine group possesses a tert-butyl substituent to serve as an NMR reporter group. The mono-capped square-antiprismatic Dy complex has a long bond (2.83 Å) to an apical N atom (pK

Identifiants

pubmed: 30861590
doi: 10.1002/chem.201900609
doi:

Types de publication

Journal Article

Langues

eng

Pagination

6212-6225

Subventions

Organisme : Engineering and Physical Sciences Research Council

Informations de copyright

© 2019 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

Auteurs

Alice C Harnden (AC)

Department of Chemistry, Durham University, South Road, Durham, DH1 3LE, UK.

Andrei S Batsanov (AS)

Department of Chemistry, Durham University, South Road, Durham, DH1 3LE, UK.

David Parker (D)

Department of Chemistry, Durham University, South Road, Durham, DH1 3LE, UK.

Classifications MeSH