Transfer of Sequence Information and Replication of Diimine Duplexes.


Journal

The Journal of organic chemistry
ISSN: 1520-6904
Titre abrégé: J Org Chem
Pays: United States
ID NLM: 2985193R

Informations de publication

Date de publication:
05 04 2019
Historique:
pubmed: 12 3 2019
medline: 3 6 2020
entrez: 12 3 2019
Statut: ppublish

Résumé

The ability of the biopolymers RNA and DNA to store and transfer information is essential to life. Herein, we demonstrate template-directed replication in a set of dimer duplexes that use reversible covalent bonds to form base-pairing interactions. Binary sequence information was encoded as a sequence of aniline and benzaldehyde subunits linked together by a diethynyl benzene backbone. These dimers formed sequence-specific, imine-linked duplexes, which could be separated and used as templates for the synthesis of daughter duplexes with identical sequences.

Identifiants

pubmed: 30855962
doi: 10.1021/acs.joc.9b00095
pmc: PMC7547894
doi:

Substances chimiques

Aniline Compounds 0
Benzaldehydes 0
Imines 0
RNA 63231-63-0
DNA 9007-49-2
aniline SIR7XX2F1K
benzaldehyde TA269SD04T

Types de publication

Journal Article Research Support, Non-U.S. Gov't

Langues

eng

Sous-ensembles de citation

IM

Pagination

3754-3761

Subventions

Organisme : Howard Hughes Medical Institute
Pays : United States

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Auteurs

Kyle R Strom (KR)

Howard Hughes Medical Institute, Department of Molecular Biology, and Center for Computational and Integrative Biology , Massachusetts General Hospital , Boston , Massachusetts 02114 , United States.

Jack W Szostak (JW)

Howard Hughes Medical Institute, Department of Molecular Biology, and Center for Computational and Integrative Biology , Massachusetts General Hospital , Boston , Massachusetts 02114 , United States.

Noam Prywes (N)

Howard Hughes Medical Institute, Department of Molecular Biology, and Center for Computational and Integrative Biology , Massachusetts General Hospital , Boston , Massachusetts 02114 , United States.

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Classifications MeSH