Fast gas chromatography-atmospheric pressure (photo)ionization mass spectrometry of polybrominated diphenylether flame retardants.

Atmospheric pressure ionization Environmental mass spectrometry Fast gas chromatography Flame retardants Photoionization Tandem mass spectrometry

Journal

Analytica chimica acta
ISSN: 1873-4324
Titre abrégé: Anal Chim Acta
Pays: Netherlands
ID NLM: 0370534

Informations de publication

Date de publication:
16 May 2019
Historique:
received: 15 10 2018
revised: 24 12 2018
accepted: 07 01 2019
entrez: 25 2 2019
pubmed: 25 2 2019
medline: 21 3 2019
Statut: ppublish

Résumé

Gas chromatography (GC) and mass spectrometry (MS) are powerful, complementary techniques for the analysis of environmental toxicants. Currently, most GC-MS instruments employ electron ionization under vacuum, but the concept of coupling GC to atmospheric pressure ionization (API) is attracting revitalized interest. API conditions are inherently compatible with a wide range of ionization techniques as well high carrier gas flows that enable fast GC separations. This study reports on the application of atmospheric pressure chemical ionization (APCI) and a custom-built photoionization (APPI) source for the GC-MS analysis of polybrominated diphenyl ethers (PBDEs), a ubiquitous class of flame retardants. Photoionization of PBDEs resulted in the abundant formation of molecular ions M

Identifiants

pubmed: 30797463
pii: S0003-2670(19)30046-7
doi: 10.1016/j.aca.2019.01.007
pmc: PMC7428865
mid: NIHMS1602460
pii:
doi:

Substances chimiques

Flame Retardants 0
Halogenated Diphenyl Ethers 0

Types de publication

Journal Article

Langues

eng

Sous-ensembles de citation

IM

Pagination

70-78

Subventions

Organisme : NICHD NIH HHS
ID : U01 HD087177
Pays : United States

Informations de copyright

Copyright © 2019. Published by Elsevier B.V.

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Auteurs

Robert A Di Lorenzo (RA)

Mouse Imaging Centre, The Hospital for Sick Children, 25 Orde Street, Toronto, ON, M5T 3H7, Canada.

Vladislav V Lobodin (VV)

National High Magnetic Field Laboratory, Florida State University, 1800 E Paul Dirac Dr., Tallahassee, FL, 32310, USA. Electronic address: Lobodin@magnet.fsu.edu.

Jack Cochran (J)

VUV Analytics, 715 Discovery Blvd. Suite 502, Cedar Park, TX, 78613, USA.

Terry Kolic (T)

Ontario Ministry of the Environment, Conservation and Parks, 125 Resources Road, Toronto, Ontario, M9P 3V6, Canada.

Sladjana Besevic (S)

Ontario Ministry of the Environment, Conservation and Parks, 125 Resources Road, Toronto, Ontario, M9P 3V6, Canada.

John G Sled (JG)

Mouse Imaging Centre, The Hospital for Sick Children, 25 Orde Street, Toronto, ON, M5T 3H7, Canada.

Eric J Reiner (EJ)

Ontario Ministry of the Environment, Conservation and Parks, 125 Resources Road, Toronto, Ontario, M9P 3V6, Canada; Department of Chemistry, University of Toronto, 80 St. George St., Toronto, ON, M5S 3H6, Canada.

Karl J Jobst (KJ)

Ontario Ministry of the Environment, Conservation and Parks, 125 Resources Road, Toronto, Ontario, M9P 3V6, Canada; Department of Chemistry and Chemical Biology, McMaster University, 1280 Main St. W., Hamilton, ON, L8S 4M1, Canada. Electronic address: Karl.Jobst@ontario.ca.

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Classifications MeSH